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This collection primarily contains outgoing letters by William Pitt, 1st Earl of Chatham; Hester Pitt, Countess of Chatham; William Pitt the Younger; and John Pitt, 2nd Earl of Chatham. Most of the letters are addressed to influential political figures such as Thomas Townshend, 1st Viscount Sydney; Henry Dundas, 1st Viscount Melville; and Count Semen Romanovich Vorontsov. The letters pertain to domestic and international political issues in Great Britain, including military conflicts in North America and Europe.

This collection is primarily made up of outgoing letters by William Pitt, 1st earl of Chatham; Hester Pitt, countess of Chatham; William Pitt the Younger; and John Pitt, 2nd earl of Chatham. Most of the letters are addressed to influential political figures such as Thomas Townshend, 1st Viscount Sydney; Henry Dundas, 1st Viscount Melville; and Count Semen Romanovich Vorontsov. The letters pertain to domestic and international political issues in Great Britain, including military conflicts in North America and Europe.

The earliest items relate to William Pitt, 1st Earl of Chatham, and his involvement in British politics in the mid-18th century. In letters to various political figures, he discussed military conflicts in Europe and North America during the Seven Years' War and other issues related to the North American colonies, such as illegal trade with French territories. Also present are 2 commissions that Pitt signed in 1760, notes on Parliamentary speeches by several politicians, and a brief poem by Pitt. In a series of letters written shortly after Pitt's death in 1778, his wife Hester Grenville Pitt and others reacted to his death. During her widowhood, Hester Grenville Pitt often wrote to banker Thomas Coutts about her sons and about other personal subjects. Letters from John Pitt, 2nd Earl of Chatham, to various recipients frequently concern his involvement in naval and other military affairs.

The outgoing letters of William Pitt the Younger comprise the bulk of the collection. He most frequently wrote to William Petty, 2nd Earl of Shelburne; Thomas Townshend, 1st Viscount Sydney; Henry Dundas, 1st Viscount Melville; Count Semen Romanovich Vorontsov of Russia; and George Rose, secretary to the Treasury under Lord Shelburne and William Pitt. Pitt discussed a multitude of subjects pertaining to Great Britain's domestic political affairs and international relations; he mentioned domestic taxation, political appointments and officeholders, legislation, the "East Indies business," and the personal affairs of the Prince of Wales. His letters also concern the Irish uprising of 1798, the French Revolutionary Wars, the Napoleonic Wars, and foreign relations with Russia. In his letter to John Fane, 10th Earl of Westmoreland, on February 7, 1801, Pitt briefly described his reasons for resigning as prime minister. Small groups of Pitt's letters to Henry Dundas, 1st Viscount Melville; Richard Wellesley, 1st Marquess Wellesley; and George Rose are housed in bound volumes. The book of letters to Wellesley contains the bookplate of Archibald Philip Primrose, 5th Earl of Rosebery, 1st Earl of Midlothian.

The Quaker Collection consists of miscellaneous letters, diaries, and documents relating to the religious and social history of the Society of Friends in America during the 18th and 19th centuries.

The Quaker collection consists of miscellaneous letters, diaries, and documents related to the religious and social history of the Society of Friends in America during the 18th and 19th centuries. These items offer insights into Quaker's daily activities and concerns, such as family life, education, and attending meetings, as well as their participation in various social reform movements, such as abolition, treatment of Native Americans, prison improvements, temperance, and pacifism. The collection also documents internal divergences of American Quakerism in the 19th century, particularly the social and doctrinal disputes that culminated in the Hicksite and Wilburite schisms.

• 1707: A manuscript copy of the death warrant of William Leddra, the last of four Quakers (including Mary Dyer) executed in Massachusetts Bay colony for their religious beliefs
• July 26, 1755: A letter from Alexander Colden to Sir William Johnson voicing frustration with Quakers who refuse to support the war effort in Pennsylvania, and an announcement of General Braddock's defeat
• August 4-12 and 17, 1761: Two accounts, one by an anonymous woman, of Quaker presence at Treaty negotiations held at Easton, Pennsylvania, between the government of Pennsylvania and the Six Nations tribes. Discussed are the negotiations, Quaker-Indian interactions, and the role of Quaker women in the Society
• [After 1770]: An account by an anonymous author of a conference with Native Americans, mostly of the Minnisink Tribe
• October 13, 1829: A letter from Phoebe Post Willis of Jericho, New York, to Isaac Post on the death of John Hicks and strife between Orthodox and Hicksite Quakers
• March 10, 1843: A letter from Ethan Foster of Westerly, Rhode Island, to Thomas B. Gould on Wilburite-Gurneyite strife in his local meeting, and the disownment of Wilbur
• [After 1863 July]: A letter describing a meeting between Abraham Lincoln and five Quaker prisoners of war, who had been forced into the Confederate army, captured by the Union, and held at Fort Delaware
• Various dates: Reports, minutes, and epistles from yearly friends meetings in America and Great Britain