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Correspondence, poems, articles, addresses, account book, and Delta Kappa Epsilon autograph book; letter book, 1883-1884, dealing mainly with prisons and jails in Michigan which Barbour inspected; scrapbook of miscellaneous clippings and scattered correspondence. Portraits and informal photos of Barbour, daguerrotypes of Barbour as a child and of his father, John Barbour, and autograph book (1860s) with portraits of members of Delta Kappa Epsilon (University of Michigan); a composite photo of the a composite photo of Michigan Constitutional Convention, 1907/1908 (with Barbour).

Librarian of University of Michigan. Correspondence, including material on library administration, collection development, opening a new library in 1883, and the exhibition of University of Michigan professor's books at the 1893 World's Fair; also family correspondence, including letters discussing travels and Civil War service of family members; and photographs.

The collection includes correspondence; files relating to his career as chief librarian of the University of Michigan; personal and biographical materials; and speeches, essays, and writings.