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The Washington & Jefferson College Student album contains carte-de-visite portraits of Jefferson College students and various other individuals, many of whom are identified. Several of the college students belonged to the fraternity Delta Tau Delta. Many photographs originated in Washington, Pennsylvania; Canonsburg, Pennsylvania; and Ann Arbor, Michigan.

The Washington & Jefferson College Student album (13cm x 18cm) contains 79 cartes-de-visite, 1 tintype, and 1 lithograph. The original brown leather cover, now detached, has a partially raised geometric design and two metal clasps; a floral design is carved into the sides of the pages. Most items are individual portraits of young men, though a few pictures of women and children are also present, including a group portrait of four women and three men. One carte-de-visite has a decorative border printed directly on the card backing.

Many of the individuals pictured signed their photographs and wrote brief notes; several of the men photographed in Washington and Canonsburg, Pennsylvania, mentioned their membership in the Delta Tau Delta fraternity. A large number of photographs are attributed to George C. Gillett of Ann Arbor, Michigan; the album contains a portrait of University of Michigan professors Alonzo Benjamin Palmer, Samuel Glasgow Armor, and Corydon L. Ford; and a lithograph of the University of Michigan campus in Ann Arbor. A number of the other portraits taken in Ann Arbor are signed by men who took courses in medicine at the University of Michigan during the 1860s. The volume includes one portrait of a young child that may have been taken postmortem and one carte-de-visite with artificial coloring.