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These albums contain photographs taken during Robert Peary's expeditions into the arctic regions. Volume 1 represents the 1897 trip to present-day Nunavut and Greenland on the ship Hope. The photographs feature arctic scenery, members of Peary's crew, the Hope, Inuit dwellings and American camps. The Inuit adults and children pictured include some of those who returned with Peary to the United States. Volume 2 represents one of the later Peary expeditions from 1905-1906, or 1908-1909. The images in this volume were removed from the original housing and are without identification. A vessel resembling Peary's ship from the later expeditions, S.S. Roosevelt, appears in several photos, as does a man resembling the Roosevelt's Captain, Robert Abram Bartlett.

Volume one contains 100 9cm x 9cm photographs taken during Robert Peary's expedition to present-day Nunavut and Greenland on the ship Hope in the summer of 1897. Each page (17cm x 29cm) contains two items; most include brief captions identifying places and people pictured. The volume's original covers are missing.

Many of the photographs feature scenery along Baffin Island in present-day Nunavut, including icebergs and glaciers; views of the Hope; small boats; Inuit boats and kayaks; Inuit huts and American tents; and natural features such as waterfalls, glaciers, and icebergs. The photographer also took pictures of Inuit adults, children, and crew members onboard the Hope; captions identify Robert Peary, his daughter Marie and her African American nurse, members of the expedition, and Inuit persons named "Kishu" and "Minnie". Kisuh may be Qisuk, and Minnie is very likely Minik, who were both taken to New York by Peary. A group photograph taken onboard ship may include Matthew Henson, Peary's African American assistant, although not identified as such. A few pictures were taken inside what appears to be a small wooden structure, and crew members occasionally posed outdoors with deer and caribou they had killed. One photograph of a "Fossil Bed" appears to have been printed from a broken glass plate negative.

Volume 2 is comprised of 92 12cm x 18cm and 10cm x 13cm photographic prints, likely taken on the Peary expedition of 1905 or later. The prints have been removed from the no longer extant original album pages, and are currently housed in a dark green ring-binder in a tan cloth sleeve measuring 34cm x 31cm. The images include scenes of northern settlements and camps; ice flows; crew-members on board ship; the hunting of a walrus, displaying a polar bear's head; men with bear cubs; and Inuit people, their dwellings, kayaks and boats. Several vessels appear including one that is likely the SS Roosevelt; also a fishing schooner; and an unidentified steamship. There are many portraits of crew members, all unidentified. Several are of a man resembling the Roosevelt's Captain, Robert Abram Bartlett.

Three magazine clippings from the mid-20th century are included that refer to Captain Bartlett.