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The Cross-Country photograph album contains photographs taken in various locations throughout the United States, including travel photographs of scenery and buildings in Washington, Colorado, Louisiana, and Massachusetts, among other states, and family photographs taken in New Hampshire, Massachusetts, and elsewhere.

The Cross-Country photograph album (26cm x 32cm, 59 pages) contains around 340 photographs taken throughout the United States between 1896 and 1907, including 15 cyanotypes and 10 panoramas. The items represent numerous printing processes in a variety of sizes. Some have captions, often providing information about the place and the date. Several reference the Gill family. The album has the title "Photographs" printed in gold on its front cover and its pages are bound with a thick string.

Many of the photographs are casual group portraits of men, women, children, and family dogs taken outdoors, often in front of large houses and cottages; some of the same individuals are present in multiple pictures. Included are a portrait of an African American woman holding a Caucasian infant (p. 1), two young boys in dress military uniforms with a collection of toy soldiers (p. 3), and a wedding party (p. 46). Some men and women are pictured golfing at Bass Rocks in Gloucester, Massachusetts. Most of the remaining images are views of landscapes, city streets, buildings, and natural scenery in locations such as Spokane, Washington; Tacoma, Washington; Lake Coeur d'Alene, Idaho; Pikes Peak, Colorado; New Orleans, Louisiana; Hampton, New Hampshire; Boston, Massachusetts; Gloucester, Massachusetts; Beacon Falls, Connecticut; and Washington, D.C. Included are a small number of commercial photographs of the area around Pikes Peak in Colorado including views by William H. Jackson. City views often feature prominent buildings and other landmarks. Other photographs show the rocky coast of New England, harbors, sailing vessels of various sizes, and large homes. Of note are a group portrait of Spokane Native Americans (p.14); views of the Tacoma waterfront (p.15); the New England coast, with aspects of the Gloucester fishing industry including a view of salted cod laid out to dry (p.24-29); pictures of Victorian home interiors (p. 20, 34, 47, 55, 56); and panoramic landscape views taken near Spokane (p. 47, 48). The album includes one print and a hand-colored collotype of the home of Senator George Turner in Spokane, Washington (inside front cover).