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The Academic Affiliations series (1945-1969; .3 lin. ft.) consists of three subseries: Detroit Institute of Arts (1945-1963), Richmond Museum of Fine Arts (1963-1965) and University of Michigan Museum of Art (1965-1969). The three subseries contain materials related to Grigaut's tenure at these institutions. The Detroit Institute of Arts subseries consists of four folders and contains typed and written correspondence, materials published by the Institute during Grigaut's tenure, memoranda regarding Grigaut's position as acting director and miscellaneous items. The Richmond Museum of Fine Arts subseries consists of four folders and contains typed and written correspondence, memoranda, an annual report and a few miscellaneous items. The University of Michigan Museum of Art subseries consists of three folders and contains memoranda, typed and written correspondence and miscellaneous items.

The Topical File series (.4 lin. ft.) contains 12 folders and consists of a variety of materials, including photographs, newspaper articles, obituaries, biographic materials and correspondence regarding Grigaut's death. There are also substantial amounts of materials related to Grigaut's estate, including correspondence, legal documents and inventory lists.