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Angell was a frequent speaker at civic and ceremonial events, high school and college commencements, to scholarly and professional organizations, religious groups, and the students and faculty of the university. The Addresses and articles series contains texts and outlines of speeches and a number of published articles, many of which originated as speeches. The addresses and article cover a wide range of topics including, education, religion, international affairs - especially in regard to China, and civic and patriotic themes. The series is arranged chronologically.

The Subject Files and Personal Papers series includes a variety of material reflecting Angell's interest and activities as well as aspects of his personal life. It includes notes and materials collected for historical research and lectures, files concerning his diplomatic missions and service on the fisheries commission, and material relating to the University of Michigan. The personal materials include several biographical sketches, a manuscript and typescript of The Reminiscences of James B. Angell and Angell's will and the inventory of his estate.