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Correspondence, poems, articles, addresses, account book, and Delta Kappa Epsilon autograph book; letter book, 1883-1884, dealing mainly with prisons and jails in Michigan which Barbour inspected; scrapbook of miscellaneous clippings and scattered correspondence. Portraits and informal photos of Barbour, daguerrotypes of Barbour as a child and of his father, John Barbour, and autograph book (1860s) with portraits of members of Delta Kappa Epsilon (University of Michigan); a composite photo of the a composite photo of Michigan Constitutional Convention, 1907/1908 (with Barbour).

Suffragist, leader of the Michigan Branch of the National Woman's Party, and candidate for the Michigan legislature in 1924. Correspondence, newspaper clippings, pamphlets, periodicals and other materials concerning her activities in the Michigan Equal Suffrage Association, the Legislative Council of Michigan Women, the National Woman's Party, and the Republican Party; and photographs.

The Grimes papers have been arranged into the following series: Correspondence; Other Papers (non-correspondence); Subject files; Bills introduced in the Michigan legislature; Newspaper clippings; Printed material; Scrapbooks; and Miscellaneous.