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The Brayton W. Smith diary includes daily entries detailing Smith's experiences as a student at Beloit Academy in Beloit, Wisconsin, and at the University of Michigan in Ann Arbor, Michigan, during 1867. His entries describe curricula, student life, studying habits, boarding houses, family matters, and his interest in baseball.

While attending Beloit Academy to prepare for college, Smith wrote of his coursework, progress in studying, struggles with exams, weather, and his relationships with other students, roommates, and boarding house proprietors. Smith also documented his activities with local religious groups, debating societies, and baseball clubs.

During vacations, Smith returned to his family who lived near Janesville, Wisconsin. He described his leisure activities, including picking berries and hunting, his struggles to continue studying, and his active involvement in local baseball, both in organized clubs and informal games among friends. Throughout the summer, Smith frequently documented information about area baseball clubs, practices, games, and tournaments.

In mid-September, Smith matriculated at the University of Michigan, and his diary includes a record of his experiences with entrance exams, tutoring, coursework, and his observations of student activities and elections. He also commented on the "University nine" baseball players, noting several of their games, and the creation of a baseball club for the freshman class.