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The Blake family correspondence is made up of incoming letters to Jonathan Blake of Warwick, Massachusetts, and New York City, and a smaller set of incoming letters to Blake's future son-in-law, Ephraim Lyon of New York City. Correspondents from New England and New York discussed daily life, education, religion, travel, and other topics.

The Blake family correspondence (140 items) includes incoming letters to Jonathan Blake of Warwick, Massachusetts, and New York City (around 115 letters), along with a smaller set of incoming letters to Blake's future son-in-law, Ephraim Lyon of New York City (around 15 items). Their outgoing correspondence makes up the remainder of the items.

Jonathan Blake's incoming correspondence, which is dated from 1825-1847, mainly consists of personal letters from his siblings and cousins, though he also received letters from other acquaintances. His family often provided news of their lives in Warwick, Massachusetts, and Northampton, Massachusetts, commenting on subjects such as education, local and family health, and religion. A brief group of letters between Jonathan Blake and his wife Mary in 1838, 1840, and 1843 concerns his attempts to persuade her to join him in Warwick, where he hoped to nurse his fragile health, though she did not wish to leave New York City. After 1847, the correspondence largely consists of incoming personal letters to Ephraim Lyon and Lyon's letters to Mary Blake before their marriage. His friends and family members reported on their social lives in Waterford, Connecticut, and on other subjects, and Lyon wrote to Blake about his romantic feelings for her and, in one letter, the possibility of moving to California to pursue his fortune (August 3, 1852).

The Divie and Joanna Bethune collection contains correspondence, religious diaries, and an autobiography pertaining to the New York couple.

The Divie and Joanna Bethune collection contains correspondence, religious diaries, and an autobiography pertaining to the New York couple.

The Correspondence series is made up of 59 incoming letters to Divie and Joanna Bethune, which primarily relate to Divie's business interests, and 1 letter by Joanna Bethune to George Duffield (February 9, 1837). Arthur Dalton of New Orleans, Louisiana, wrote the bulk of the early correspondence, discussing the local tobacco trade and ships' movements near the city. Divie Bethune & Co. received letters from Thomas Masters about financial affairs in Liverpool and London, England. Personal letters include letters between members of the Bethune family, such as a letter from Joanna Bethune to her daughter Isabella, which alludes to the possibility of Canadian annexation (January 6, 1850).

The 22-volume Diaries series comprises the bulk of the collection, and contains material written by both Divie and Joanna Bethune. Divie Bethune filled the first 17 volumes with devotional prayers, religious poetry, hymns, and occasional daily diary entries. Each of these volumes has an identical inscription. Joanna Bethune kept 6 diaries after her husband's death, in which she reflected upon her emotions and wrote about her charity work and religious life.

Joanna Bethune's Autobiography, written in 1814, concerns her early life, emphasizing her religious conversion and religious convictions.